Anisotropy of magnetic interactions and symmetry of the order parameter in unconventional superconductor Sr2RuO4

Author(s)
Bongjae Kim, Sergii Khmelevskyi, Igor I. Mazin, Daniel F. Agterberg, Cesare Franchini
Abstract

Sr2RuO4 is the best candidate for spin-triplet superconductivity, an unusual and elusive superconducting state of fundamental importance. In the last three decades, Sr2RuO4 has been very carefully studied and despite its apparent simplicity when compared with strongly correlated high-T c cuprates, for which the pairing symmetry is understood, there is no scenario that can explain all the major experimental observations, a conundrum that has generated tremendous interest. Here, we present a density-functional-based analysis of magnetic interactions in Sr2RuO4 and discuss the role of magnetic anisotropy in its unconventional superconductivity. Our goal is twofold. First, we access the possibility of the superconducting order parameter rotation in an external magnetic field of 200 Oe, and conclude that the spin–orbit interaction in this material is several orders of magnitude too strong to be consistent with this hypothesis. Thus, the observed invariance of the Knight shift across T c has no plausible explanation, and casts doubt on using the Knight shift as an ultimate litmus paper for the pairing symmetry. Second, we propose a quantitative double-exchange-like model for combining itinerant fermions with an anisotropic Heisenberg magnetic Hamiltonian. This model is complementary to the Hubbard-model-based calculations published so far, and forms an alternative framework for exploring superconducting symmetry in Sr2RuO4. As an example, we use this model to analyze the degeneracy between various p-triplet states in the simplest mean-field approximation, and show that it splits into a single and two doublets with the ground state defined by the competition between the “Ising” and “compass” anisotropic terms.

Organisation(s)
Computational Materials Physics
External organisation(s)
U.S. Naval Research Laboratory, University of Wisconsin, Milwaukee
Journal
npj Quantum Materials
Volume
2
No. of pages
7
ISSN
2397-4648
DOI
https://doi.org/10.1038/s41535-017-0041-8
Publication date
2017
Peer reviewed
Yes
Austrian Fields of Science 2012
103018 Materials physics
Keywords
ASJC Scopus subject areas
Electronic, Optical and Magnetic Materials, Condensed Matter Physics
Portal url
https://ucris.univie.ac.at/portal/en/publications/anisotropy-of-magnetic-interactions-and-symmetry-of-the-order-parameter-in-unconventional-superconductor-sr2ruo4(6a440762-1af9-435a-80e1-b30da3c78ebd).html