The versatile size analyzing nuclei counter (vSANC)
- Author(s)
- Tamara Pinterich, Aron Vrtala, Merzuk Kaltak, Juha Kangasluoma, Katrianne Lehtipalo, Tuukka Petaja, Paul M. Winkler, Markku Kulmala, Paul E. Wagner
- Abstract
We present a new field-deployable expansion chamber condensation particle counter-the versatile size analyzing nuclei counter (vSANC). The measuring principle, which was adopted from the classical SANC, was optimized regarding ranges of operating temperatures (-20 degrees C to +40 degrees C/, inlet gas pressures (0.2-1.2 bar), inlet flow rates (1.6-9 l/min) and condensing liquids (alcohols, alcanes, water, etc.), all of which make vSANC applicable to a wide variety of environments. Precision determination of vapor supersaturation ratios allows estimating neutral cluster sizes without prior electrical-mobility based classification of the sample. Additionally, absolute number concentrations ranging from 10(2) to 10(7)cm(-3) can be measured without referring to external calibration standards. This enables size-resolved number concentration measurements of nanoparticles. Laboratory studies using n-propanol as condensing liquid demonstrated that charged (NH4)(2)SO4 and WOx particles as small as 1.5 nm can be counted with an efficiency of 10%. Furthermore, we observed an increase in counting efficiency of charged WOx particles by about 50% when lowering vSANC's chamber and saturator temperatures from 23 degrees C and 25 degrees C to 13 degrees C and 15 degrees C, respectively. During spring 2014, the vSANC was operated at the SMEAR II station in Finland where the formation and growth of atmospheric clusters was investigated. Atmospheric new particle formation (NPF) was observed only when vSANC's operating temperatures (13 degrees C and 15 degrees C) were close to the ambient air temperature (about 5 degrees C-15 degrees C). Diurnal concentration evolution measured with the vSANC was compared with data from a differential mobility particle sizer (DMPS) and a nano-condensation nucleus counter (nCNC, Airmodus A11). vSANC detected the NPF signal 2-3 h before the DMPS in agreement with the nCNC; however, a continuously present pool of highly concentrated neutral clusters in the sub-3 nm diameter range could not be confirmed during these measurements.
- Organisation(s)
- Aerosol Physics and Environmental Physics, Computational Materials Physics
- External organisation(s)
- Brookhaven National Laboratory, State University of New York, Stony Brook, University of Helsinki, Paul Scherrer Institute
- Journal
- Aerosol Science and Technology
- Volume
- 50
- Pages
- 947-958
- No. of pages
- 12
- ISSN
- 0278-6826
- DOI
- https://doi.org/10.1080/02786826.2016.1210783
- Publication date
- 2016
- Peer reviewed
- Yes
- Austrian Fields of Science 2012
- 103037 Environmental physics, 103039 Aerosol physics
- Keywords
- ASJC Scopus subject areas
- Pollution, Materials Science(all), Environmental Chemistry
- Portal url
- https://ucris.univie.ac.at/portal/en/publications/the-versatile-size-analyzing-nuclei-counter-vsanc(ca3e0c2b-ed44-4472-8370-daf50704036f).html