Revisiting Mn-doped Ge using the Heyd-Scuseria-Ernzerhof hybrid functional

Author(s)
Alessandro Stroppa, Georg Kresse, A Continenza
Abstract

We perform a comparative ab initio study of Mn-doped germanium semiconductor using the Perdew-Burke-Ernzerhof exchange-correlation functional, density functional theory (DFT) + U, and Heyd-Scuseria-Ernzerhof hybrid functional (HSE). We show that the HSE functional is able to correctly account for the relevant ground-state properties of the host matrix as well as of the Mn-doped semiconductor. Although the DFT + U and the HSE description are very similar, some differences still remain. In particular, the half metallicity is lost using DFT + U when a suitable U value, tuned to recover the photoemission spectra, is employed. For comparison, we also discuss the case of Mn in silicon.

Organisation(s)
Computational Materials Physics
External organisation(s)
Università degli Studi dell’Aquila
Journal
Physical Review B
Volume
83
No. of pages
5
ISSN
1098-0121
DOI
https://doi.org/10.1103/PhysRevB.83.085201
Publication date
2011
Peer reviewed
Yes
Austrian Fields of Science 2012
103018 Materials physics
Portal url
https://ucrisportal.univie.ac.at/en/publications/revisiting-mndoped-ge-using-the-heydscuseriaernzerhof-hybrid-functional(2db7affb-45cf-4d3d-8537-74d2db488497).html