Adsorption of small molecules on the [Zn-Zn]2+linkage in zeolite. A DFT study of ferrierite

Author(s)
Lubomir Benco
Abstract

In zeolites monovalent Zn(I) forms a sub-nano particles [Zn-Zn]2+ stabilized in rings of the zeolite framework, which exhibit interesting catalytic properties. This work reports on adsorption properties of [Zn-Zn](2+) particles in zeolite ferrierite investigated for a set of probing diatomic (N-2, O-2, H-2, CO, NO) and triatomic (CO2, N2O, NO2, H2O) molecules using dispersion-corrected DFT. Three [Zn-Zn]2+ sites are compared differing in the location and stability. On all sites molecules form physisorbed clusters with the molecule connected on-top of the Zn Zn linkage. In physisorbed clusters adsorption induces only slight change of bonding and the geometry of the Zn-Zn linkage. Some molecules can form stable chemisorbed clusters in which the molecule is integrated between two Zn+ cations. The sandwich-like chemisorption causes pronounced changes of bonding and can lead to the transfer of the electron density between two Zn+ cations and to a change of the oxidation state. The knowledge of bonding of small molecules can help understanding of the mechanism of conversion reactions catalyzed by sub-nano [Zn-Zn] particles

Organisation(s)
Computational Materials Physics
Journal
Surface Science
Volume
656
Pages
115-125
No. of pages
11
ISSN
0039-6028
DOI
https://doi.org/10.1016/j.susc.2016.10.011
Publication date
02-2017
Peer reviewed
Yes
Austrian Fields of Science 2012
103025 Quantum mechanics, 103036 Theoretical physics, 103015 Condensed matter, 103009 Solid state physics
Keywords
ASJC Scopus subject areas
Condensed Matter Physics, Materials Chemistry, Surfaces, Coatings and Films, Surfaces and Interfaces
Portal url
https://ucrisportal.univie.ac.at/en/publications/b7667da7-8ab2-46fa-883a-721b471fd28e